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6
TableofContents
3.8.3.CaseofZirconia-basedMaterials.................
3.8.4.DefectStructureofYSZ........................
3.9.Debye-HückelDefectModel...........................
3.9.1.CO
1-yOCase..................................
3.10.ClusterModel.......................................
3.10.1.DefectClusteringintheWustitePhase.............
3.11.CrystallographicShearing.............................
3.12.DefectStructureofTitaniumDioxide....................
3.12.1.ExtendedDefectsinTiO
2
.......................
3.13.HydrogenDefects....................................
Acknowledgements.......................................
References..............................................
67
72
73
73
77
77
80
81
85
86
87
87
4.
Self-PolarizationofFerroelectricThinFilmsandItsInfluence
ontheFilmProperties...................................
92
4.1.Introduction........................................
93
4.2.FreeEnergyFunctional...............................
94
4.3.RenormalizedFreeEnergyandPropertiesforOneComponent
PolarizationP=P
Z...................................
96
4.4.TheInfluenceofBuilt-inElectricFieldonthePropertiesof
FerroelectricThinFilmsfortheCaseP=P
Z...............
99
4.5.PhaseDiagramswithElectretStateandPropertiesfortheCase
ofThreePolarizationComponents.......................103
4.6.ComparisonwithExperimentandSummaryofSec.5Results.114
Conclusion..............................................117
References..............................................118
5.
LatticeDynamicsofPerovskiteOxides....................120
5.1.Introduction........................................120
5.2.EarlyAttemptstoModelFerroelectricPerovskites..........121
5.3.PolarizabilityEfectsinPerovskites......................124
5.4.ThePolarizabilityModelforPerovskites..................126
5.5.ApplicationsoftheModel.............................131
5.6.PrecursorEfectstothePhaseTransitions.................137
Conclusions.............................................146
References..............................................147
6.
MetrologyandMeasurementTechniques..................151
6.1.ElectricalPropertiesofNanoscaleSolids..................151
6.1.1.MeasurementofElectricalandMagneticMaterial
Properties....................................152
